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Beilstein J. Org. Chem. 2017, 13, 1879–1892, doi:10.3762/bjoc.13.183
Graphical Abstract
Figure 1: β-Cyclodextrin- and adamantyl-substituted poly(acrylate)s PAAβ-CDen, PAAADen, PAAADhn, and PAAADddn...
Figure 2: ITC data for the PAAβ-CDen/PAAADen, system obtained in aqueous Na2HPO4/KH2PO4 pH 7.0 buffer at I = ...
Figure 3: ITC data for the PAAβ-CDen/PAAADddn system obtained in aqueous Na2HPO4/KH2PO4 pH 7.0 buffer at I = ...
Figure 4: Representation of ditopic complexation of an ADddn substituent of PAAADddn, by two β-CDen substitue...
Figure 5: 2D NOESY 1H NMR spectrum of 0.44 wt % PAAβ-CDen ([β-CDen] = 2.0 × 10−3 mol dm−3) and 0.60 wt % PAAA...
Figure 6: (a) Molar absorbance variation of 1.5 cm3 of a EO solution ([EO] = 2.00 × 10−5 mol dm−3) with 20 se...
Figure 7: (a) Molar absorbance variation of 1.5 cm3 of a EO solution ([EO] = 2.00 × 10−5 mol dm−3) with 20 se...
Figure 8: Speciation plot with [β-CDen]total = 100% for the PAAβ-CDen/PAAADhn/EO system.
Figure 9: 2D NOESY 1H NMR spectrum of MR ([MR] = 2.0 × 10−3 mol dm−3) in solution with PAAβ-CDen (0.78 wt %, ...
Figure 10: Viscosity variations at a 0.03 s−1 shear rate of 1.14 wt % PAAβ-CDen/PAAADen, 1.18 wt % PAAβ-CDen/P...
Figure 11: Representation of dye complexation in the PAAβ-CDen/PAAADen and PAAβ-CDen/PAAADhn networks.
Figure 12: Release profiles for EO (i), MO (ii) and MR (iii) from aqueous (a) Na2HPO4/KH2PO4 buffer alone, (b)...
Beilstein J. Org. Chem. 2015, 11, 2370–2387, doi:10.3762/bjoc.11.259
Figure 1: Biocatalytic routes for conversion of CO2 into compounds with carbon in the reduced oxidation state...
Figure 2: Carbonic anhydrase-catalysed rapid interconversion of CO2 and HCO3− in living systems.
Scheme 1: The Calvin cycle for fixation of CO2 with RuBisCO.
Scheme 2: The reductive TCA cycle with CO2 fixation enzymes designated.
Scheme 3: The Wood–Ljungdahl pathway for generation of acetyl-CoA through reduction of CO2 to formate and CO....
Scheme 4: The acyl-CoA carboxylase pathways for autotrophic CO2 fixation. ACC: acetyl-CoA/propionyl-CoA carbo...
Figure 3: RuBisCO CO2-fixing bypass installed in E. coli and S. cerevisiae to increase carbon flux toward pro...
Scheme 5: Integrated biocatalytic system for carboxylation of phosphoenolpyruvate (19), using PEPC and carbon...
Scheme 6: PEPC and pyruvate carboxylase catalysed carboxylation of pyruvate backbone for the generation of ox...
Scheme 7: Decarboxylase catalysed carboxylation of (a) phenol derivatives, (b) indole and (c) pyrrole.
Figure 4: Formate dehydrogenase (FDH) catalysed reversible reduction of CO2 to formate with electron donor re...
Figure 5: Sequential generation of formate, formaldehyde and methanol from CO2 using reducing equivalents sou...
Figure 6: Hydrogen storage as formic acid through biocatalytic hydrogenation of CO2 and subsequent on-demand ...
Figure 7: Schematic showing required flow of reducing equivalents for CO2 fixation through biotechnological a...